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Proceedings Paper

Ultrafast magnetism as seen by x-rays
Author(s): Ilie Radu; Kadir Vahaplar; Christian Stamm; Torsten Kachel; Niko Pontius; Florin Radu; Radu Abrudan; Hermann Dürr; Thomas Ostler; Joe Barker; Richard Evans; Roy Chantrell; Arata Tsukamoto; Akiyoshi Itoh; Andrei Kirilyuk; Theo Rasing; Alexey Kimel
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Paper Abstract

Revealing the ultimate speed limit at which magnetic order can be controlled, is a fundamental challenge of modern magnetism having far reaching implications for magnetic recording industry. Exchange interaction is the strongest force in magnetism, being responsible for ferromagnetic or antiferromagnetic spin order. How do spins react after being optically perturbed on an ultrashort timescales pertinent to the characteristic time of the exchange interaction? Here we demonstrate that femtosecond measurements of X-ray magnetic circular dichroism provide revolutionary new insights into the problem of ultrafast magnetism. In particular, we show that upon femtosecond optical excitation the ultrafast spin reversal of Gd(FeCo) - a material with antiferromagnetic coupling of spins - occurs via a transient ferromagnetic state. The latter one emerges due to different dynamics of Gd and Fe magnetic moments: Gd switches within 1.5 ps while it takes only 300 fs for Fe. Thus, by using a single fs laser pulse one can force the spin system to evolve via an energetically unfavorable way and temporary switch from an antiferromagnetic to ferromagnetic type of ordering. These observations supported by atomistic simulations, present a novel concept of manipulating magnetic order on different classes of magnetic materials on timescales of the exchange interaction.

Paper Details

Date Published: 20 February 2012
PDF: 9 pages
Proc. SPIE 8260, Ultrafast Phenomena and Nanophotonics XVI, 82601M (20 February 2012); doi: 10.1117/12.907433
Show Author Affiliations
Ilie Radu, Radboud Univ. Nijmegen (Netherlands)
Helmholtz-Zentrum Berlin (Germany)
Kadir Vahaplar, Radboud Univ. Nijmegen (Netherlands)
Christian Stamm, Helmholtz-Zentrum Berlin (Germany)
Torsten Kachel, Helmholtz-Zentrum Berlin (Germany)
Niko Pontius, Helmholtz-Zentrum Berlin (Germany)
Florin Radu, Helmholtz-Zentrum Berlin (Germany)
Radu Abrudan, Ruhr-Univ. Bochum (Germany)
Hermann Dürr, Helmholtz-Zentrum Berlin (Germany)
SLAC National Accelerator Lab. (United States)
Thomas Ostler, The Univ. of York (United Kingdom)
Joe Barker, The Univ. of York (United Kingdom)
Richard Evans, The Univ. of York (United Kingdom)
Roy Chantrell, The Univ. of York (United Kingdom)
Arata Tsukamoto, Nihon Univ. (Japan)
Akiyoshi Itoh, Nihon Univ. (Japan)
Andrei Kirilyuk, Radboud Univ. Nijmegen (Netherlands)
Theo Rasing, Radboud Univ. Nijmegen (Netherlands)
Alexey Kimel, Radboud Univ. Nijmegen (Netherlands)

Published in SPIE Proceedings Vol. 8260:
Ultrafast Phenomena and Nanophotonics XVI
Markus Betz; Abdulhakem Y. Elezzabi; Jin-Joo Song; Kong-Thon Tsen, Editor(s)

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