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Optimizing CARS signal using coherent control methods
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Paper Abstract

We demonstrate the adiabatic passage based method to maximize CARS coherence and present numerical results of the roof scheme implementation without making an assumption of adiabatic elimination of detuned excited electronic states. Also we analyze influence of fast decoherence in the molecular samples on the results of proposed scheme. It is shown that the adiabatic method allows achieving chemical sensitivity with high resolution and can be used to obtain CARS signal with efficiently suppressed background in molecular systems with coherence times of several hundred of femtoseconds.

Paper Details

Date Published: 25 February 2009
PDF: 8 pages
Proc. SPIE 7183, Multiphoton Microscopy in the Biomedical Sciences IX, 71830Q (25 February 2009); doi: 10.1117/12.809691
Show Author Affiliations
Vladimir S. Malinovsky, MagiQ Technologies, Inc. (United States)

Published in SPIE Proceedings Vol. 7183:
Multiphoton Microscopy in the Biomedical Sciences IX
Ammasi Periasamy; Peter T. C. So, Editor(s)

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