We rejort on the experimental realisation of time-resolved coincident Coulomb explosion imaging of H2-fragmentation in 10¹⁴ W/cm² laser fields. Combining a high-resolution 'reaction microscope' and a fs pump-probe setup, we map the motion of wave packets dissociating via one- or two-photon channels, respectively, and observe two region of enhanced ionization in accordance with earlier theoretical predictions. The long-term interferometric stability of our system allows us to extend pump-probe experiments into the region of overlapping pulses, which offers new possibilities for the manipulation of ultrafast molecular fragmentation dynamics.

Date Published: 22 May 2006
PDF: 11 pages
Proc. SPIE 6256, ICONO 2005: Ultrafast Phenomena and Physics of Superintense Laser Fields; Quantum and Atom Optics; Engineering of Quantum Information, 62560C (22 May 2006); doi: 10.1117/12.682358

Published in SPIE Proceedings Vol. 6256:
ICONO 2005: Ultrafast Phenomena and Physics of Superintense Laser Fields; Quantum and Atom Optics; Engineering of Quantum Information
Hans A. Bachor; Andre D. Bandrauk; Paul B. Corkum; Markus Drescher; Mikhail Fedorov; Serge Haroche; Sergei Kilin; Alexander Sergienko, Editor(s)