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Proceedings Paper

Discrete spectrum of anti-Stokes emission from metal particle-adsorbate complexes in a microcavity
Author(s): Vladimir P. Drachev; Won-Tae Kim; Eldar Nailevich Khaliullin; Fedda Al-Zoubi; Viktor A. Podolskiy; Vladimir P. Safonov; Vladimir M. Shalaev; Robert L. Armstrong
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Paper Abstract

This report presents the discovery of greatly enhanced, broad-range, multiphoton excited emission from Ag aggregate- adsorbate complexes seeded into a cylindrical microcavity. The emission spectrum contains descrete peaks spanning the wavelength range from the 632 nm HeNe laser exciting wavelength down to 200 nm. Observation of multiphoton processes at the low exciting light intensity (20 W/cm2) became possible due to using a fractal-microcavity composite, where coupling the localized plasmon modes in fractal aggregates with microcavity resonances is provided. The important role of the multiphoton resonant transitions between discrete states of a finite-size metal particle in enhanced local fields is shown. Analysis, based on the model of a spherical potential well, shows that the observed spectra contain fingerprints of the quantum size effect.

Paper Details

Date Published: 29 May 2002
PDF: 10 pages
Proc. SPIE 4748, ICONO 2001: Fundamental Aspects of Laser-Matter Interaction and Physics of Nanostructures, (29 May 2002); doi: 10.1117/12.468975
Show Author Affiliations
Vladimir P. Drachev, Institute of Semiconductor Physics (Russia)
Won-Tae Kim, New Mexico State Univ. (United States)
Eldar Nailevich Khaliullin, New Mexico State Univ. (United States)
Fedda Al-Zoubi, New Mexico State Univ. (United States)
Viktor A. Podolskiy, New Mexico State Univ. (United States)
Vladimir P. Safonov, Institute of Automation and Electrometry (Russia)
Vladimir M. Shalaev, New Mexico State Univ. (United States)
Robert L. Armstrong, New Mexico State Univ. (United States)

Published in SPIE Proceedings Vol. 4748:
ICONO 2001: Fundamental Aspects of Laser-Matter Interaction and Physics of Nanostructures
Anatoly V. Andreev; Pavel A. Apanasevich; Vladimir I. Emel'yanov; Alexander P. Nizovtsev, Editor(s)

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