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Proceedings Paper

Subpicosecond radiolysis by means of terawatt laser wakefield accelerator
Author(s): Dmitri A. Oulianov; Oleg J. Korovyanko; Robert A. Crowell; David J. Gosztola; Ilya A. Shkrob; Roberto C. Rey-de-Castro; Christopher G. Elles
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Paper Abstract

A novel subpicosecond pulse radiolysis experimental system has been developed in Terawatt Ultrafast High Field Facility (TUHFF) at Argonne National Laboratory. TUHFF houses a 20 TW Ti:sapphire laser system that generates 2.5 nC sub-picosecond pulses of 4-25 MeV electrons at 10 Hz using laser wakefield acceleration. The system has been optimized for chemical studies. The subpicosecond electron pulses were used to generate hydrated electrons in pulse radiolysis of liquid water. Preliminary transient absorption spectroscopy data with picosecond resolution is presented.

Paper Details

Date Published: 23 February 2006
PDF: 8 pages
Proc. SPIE 6101, Laser Beam Control and Applications, 610126 (23 February 2006); doi: 10.1117/12.675463
Show Author Affiliations
Dmitri A. Oulianov, Argonne National Lab. (United States)
Oleg J. Korovyanko, Argonne National Lab. (United States)
Robert A. Crowell, Argonne National Lab. (United States)
David J. Gosztola, Argonne National Lab. (United States)
Ilya A. Shkrob, Argonne National Lab. (United States)
Roberto C. Rey-de-Castro, Argonne National Lab. (United States)
Christopher G. Elles, Argonne National Lab. (United States)


Published in SPIE Proceedings Vol. 6101:
Laser Beam Control and Applications
Steven J. Davis; Alexis V. Kudryashov; Adolf Giesen; Detlef Nickel; Michael C. Heaven; Alan H. Paxton; Vladimir S. Ilchenko; J. Thomas Schriempf, Editor(s)

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