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Proceedings Paper

Theoretical description of SHG by fullerene film on dielectric surface
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Paper Abstract

The first hyperpolarizability (HP) of ullerene on the silica substructure, modeled by β-quartz layers, is calculated in the framework of the semi-empirical version of the time-dependent Hartree-Fock theory. The induced by the substrate orthogonal to the surface component of β-vector invariant is of the same order as in the 'push-pull' organic molecules with the expressed nonlinear optical properties. Just this component is responsible for generation of the second harmonic according to Hoshi and coauthors.

Paper Details

Date Published: 10 November 2003
PDF: 7 pages
Proc. SPIE 5212, Linear and Nonlinear Optics of Organic Materials III, (10 November 2003); doi: 10.1117/12.504614
Show Author Affiliations
Mikhail M. Mestechkin, Consultant (United States)
Gene Whyman, Institute of Physical-Organic and Coal Chemistry (Ukraine)

Published in SPIE Proceedings Vol. 5212:
Linear and Nonlinear Optics of Organic Materials III
Mark G. Kuzyk; Manfred Eich; Robert A. Norwood, Editor(s)

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