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Proceedings Paper

Optical coherence spectroscopy in solution: determining the system-bath correlation function
Author(s): Lewis D. Book; David C. Arnett; Norbert F. Scherer
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Paper Abstract

We present a method to determine system-bath correlation functions from third order optical coherence measurements. The importance of these correlation functions for understanding solvation dynamics is explained. A physical argument is made to explain why one coherence measurement, the photon echo peak shift, should strongly reflect system- bath dynamics. Finally, this method is applied to the system of bacteriochlorophyll in tetrahydrofuran solution.

Paper Details

Date Published: 24 April 1998
PDF: 9 pages
Proc. SPIE 3273, Laser Techniques for Condensed-Phase and Biological Systems, (24 April 1998); doi: 10.1117/12.306117
Show Author Affiliations
Lewis D. Book, Univ. of Chicago (United States)
David C. Arnett, Pacific Northwest National Labs. (United States)
Norbert F. Scherer, Univ. of Chicago (United States)


Published in SPIE Proceedings Vol. 3273:
Laser Techniques for Condensed-Phase and Biological Systems
Norbert F. Scherer; Janice M. Hicks, Editor(s)

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