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Proceedings Paper

Conjugation in three dimensions to enhance NLO susceptibilities
Author(s): Carl W. Dirk; Ou Xie
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Paper Abstract

We show, using AMPAC (Semichem, Inc.) AMI calculations of extended cyclophane structures that the third order polarization displays significant large magnitude negative Finite-Field (gamma) (0)s. Magnitudes as large as -85,000 X 10-36 esu are calculated. Anticipated significant linear loss issues are not addressed, though no effort has yet been made to optimize ether for maximum magnitude (gamma) or minimum magnitude linear loss structure. It is expected that such a systematic theoretical and experimental optimization of molecules should lead to materials possessing unprecedented magnitudes of (gamma) , and possibly with sufficiently low loss to be practical.

Paper Details

Date Published: 1 November 1996
PDF: 6 pages
Proc. SPIE 2852, Nonlinear Optical Properties of Organic Materials IX, (1 November 1996); doi: 10.1117/12.256185
Show Author Affiliations
Carl W. Dirk, Univ. of Texas/El Paso (United States)
Ou Xie, Univ. of Texas/El Paso (United States)

Published in SPIE Proceedings Vol. 2852:
Nonlinear Optical Properties of Organic Materials IX
Gustaaf R. Moehlmann, Editor(s)

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