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Nonlinear spectroscopy in perovskite quantum dots
Author(s): Gabriel Nagamine; Luiz Gustavo Bonato; Juan A. Castañeda; Emre Yassitepe; Ana F. Nogueira; Carlos H. Brito Cruz; Lazaro A. Padilha
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Paper Abstract

Since the first reports of their successful synthesis in 2015, all-inorganic perovskite quantum dots (PQDs), emerged as promising material for lighting applications. Despite their unique optical properties, to date, PQDs based LEDs and lasing media operation is still far from ideal. One of the limiting factors is the strong Coulomb interaction, which contributes to nonradiative decay processes. Here, we discuss in detail the multiexciton interactions in PQDs based on their size dependence. We expand on their nonlinear optical properties, focusing on the two-photon absorption characteristics, showing results for two-photon pumped amplified stimulated emission, suggesting that these materials may be promising for two-photon pumped lasers.

Paper Details

Date Published: 8 May 2018
PDF: 7 pages
Proc. SPIE 10638, Ultrafast Bandgap Photonics III, 106380K (8 May 2018); doi: 10.1117/12.2305001
Show Author Affiliations
Gabriel Nagamine, Univ. Estadual de Campinas (Brazil)
Luiz Gustavo Bonato, Univ. Estadual de Campinas (Brazil)
Juan A. Castañeda, Univ. Estadual de Campinas (Brazil)
Emre Yassitepe, Univ. Estadual de Campinas (Brazil)
Ana F. Nogueira, Univ. Estadual de Campinas (Brazil)
Carlos H. Brito Cruz, Univ. Estadual de Campinas (Brazil)
Lazaro A. Padilha, Univ. Estadual de Campinas (Brazil)


Published in SPIE Proceedings Vol. 10638:
Ultrafast Bandgap Photonics III
Michael K. Rafailov, Editor(s)

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