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Proceedings Paper

Polarized and asymmetric emission of single colloidal nanoplatelets (Conference Presentation)
Author(s): Fu Feng; Thu Loan N'Guyen; Michel Nasilowski; Clotilde M. Lethiec; Benoit Dubertret; Laurent Coolen; Agnès Maître

Paper Abstract

Efficient coupling of nanoemitters to photonic or plasmonic structures requires the control of the orientation of the emitting dipoles. Nevertheless controlling the dipole orientation remains an experimental challenge. Many experiments rely on the realization of numerous samples, in order to be able to statistically get a well aligned dipole to realize an efficient coupling to a nanostructure. In order to avoid these statistical trials, the knowledge of the nature of the emitter and its orientation is crucial for a deterministical approach. We developed a method [1],[2] relying on the combination of polarimetric measurement and emission diagram which gives fine information both on the emitting dipolar transition involved and on the dipolar orientation We analyse by this method square and rectangle single colloidal CdSe/CdS nanoplatetelets. We demonstrate that their emission can be described by just by two orthogonal dipoles lying in the plane of the platelets. More surprisingly the emission of the square nanoplatelets is not polarised whereas the rectangle one is. We demonstrate that this polarized emission is due to the rectangular shape anisotropy by a dielectric effect. [1] C. Lethiec, et al, Three-dimensional orientation measurement of a single fluorescent nanoemitter by polarization analysis, Phys. Rev. X 4, 021037 (2014), [2] C. Lethiec et al, Polarimetry-based analysis of dipolar transitions of single colloidal CdSe/CdS dot-inrods, New Journal of Physics 16, 093014 (2014) [3] S. Ithurria et al, colloidal nanoplatelets with 2 dimensional electronic structure, Nature Materials 10, 936 (2011)

Paper Details

Date Published: 28 April 2017
PDF: 1 pages
Proc. SPIE 10114, Quantum Dots and Nanostructures: Growth, Characterization, and Modeling XIV, 101140D (28 April 2017); doi: 10.1117/12.2255041
Show Author Affiliations
Fu Feng, Univ. Pierre et Marie Curie (France)
Thu Loan N'Guyen, Univ. Pierre et Marie Curie (France)
Michel Nasilowski, Univ. Pierre et Marie Curie (France)
Clotilde M. Lethiec, The Univ. of Chicago (United States)
Benoit Dubertret, Ecole Supérieure de Physique et de Chimie Industrielles de la Ville de Paris (France)
Laurent Coolen, Univ. Pierre et Marie Curie (France)
Agnès Maître, Univ. Pierre et Marie Curie (France)

Published in SPIE Proceedings Vol. 10114:
Quantum Dots and Nanostructures: Growth, Characterization, and Modeling XIV
Diana L. Huffaker; Holger Eisele, Editor(s)

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