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Proceedings Paper

Asymptotically exact analytical solution of the problem of vibrational quantum beats in molecular electronic transitions
Author(s): Yuri T. Mazurenko
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Paper Abstract

In order to calculate the characteristics of vibrational quantum beats we use the Heisenberg (time-domain) approach to the nonlinear properties of vibronic spectra. While using this approach, the intensity of emission may be expressed as the convolution-type integral that contains the nonlinear-response function. To evaluate this integral the Laplace method is applied. In so doing the value of the Stokes shift is used as a natural great parameter. This allowed the simple expressions describing the manifestations of vibrational quantum beats to be obtained.

Paper Details

Date Published: 17 June 1993
PDF: 11 pages
Proc. SPIE 1921, Laser Spectroscopy of Biomolecules, (17 June 1993); doi: 10.1117/12.146151
Show Author Affiliations
Yuri T. Mazurenko, S. I. Vavilov State Optical Institute (United States)

Published in SPIE Proceedings Vol. 1921:
Laser Spectroscopy of Biomolecules
Jouko E. Korppi-Tommola, Editor(s)

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